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Two-Dimensional Vibrational-Electronic Spectroscopy: The Design and Development of a Novel Multidimensional Spectroscopic Technique to Directly Measure Coherent Coupling Between Vibrational and Electronic Degrees of Freedom
Two-dimensional vibrational-electronic (2D VE) spectroscopy fulfills the need for a direct measure of how vibrational motions effect electron transfer. This third-order Fourier transform technique probes electronic transitions that occur after excitation of an infrared (IR) pump. The information contained within a 2D VE ...